РЕКОНСТРУКЦІЯ ПРОКАЛЕНИХ Zn –Al ШАРУВАТИХ ПОДВІЙНИХ ГІДРОКСИДІВ ПІД ЧАС АДСОРБЦІЇ ТЕТРАЦИКЛІНУ

G. M. Starukh, O. I. Oranska, S. I. Levytska

Анотація


Zn-Al змішані оксиди, які містили ZnO різного ступеня кристалічності, були отримані при прокалюванні Zn-Al шаруватих подвійних гідроксидів (ШПГ). Реконструкція прокалених Zn-Al ШПГ проводилась при перемішуванні їх водних суспензій. Було показано, що здатність Zn-Al ШПГ відновлювати шарувату структуру шляхом гідратації змішаних оксидів, залежить від ступеня кристалічності ZnO. Часткова реконструкція Zn-Al шаруватої структури відбувається в розчинах тетрацикліну незалежно від ступеня кристалічності ZnO в прокалених ШПГ. Прокалені ШПГ проявляють високу адсорбційну здатність до тетрацикліну

Ключові слова


Zn-Al шаруваті подвійні гідроксиди, реконструкція шаруватої структури, тетрациклін, адсорбція

Повний текст:

PDF (English)

Посилання


Cavani F.,Trifirò F., Vaccari A.Hydrotalcite-type anionic clays: Preparation, properties and applications // Catal. Today. – 1991 – Vol. 11, N 2. – P. 173-301. http://dx.doi.org/10.1016/0920-5861(91)80068-K

Xu R., Pang W., Huo Q. Modern Inorganic Synthetic Chemistry [Assembly chemistry of anion-intercalated layered materials]. Amsterdam, Elsevier, 2011. 590p.

Abelló S., Medina F., Tichit D., Pérez-Ramírez J., Groen J., Sueiras J., Salagre P., Cesteros Y.Aldol Condensations Over Reconstructed Mg–Al Hydrotalcites: Structure–Activity Relationships Related to the Rehydration Method // Chem. Eur. J. – 2005 – Vol. 11, N 2. – P. 728-739. http://dx.doi.org/10.1002/chem.200400409.

Del Hoyo C.Layered double hydroxides and human health: An overview // Appl. Clay Sci. – 2007 – Vol. 36, N 1-3. – P. 103-121. http://dx.doi.org/10.1016/j.clay.2006.06.010

Vaccari A.Clays and catalysis: a promising future // Appl. Clay Sci. – 1999. – Vol. 14, N 3. – P.161–198.

Goh K., Lim T., Gong Z. Application of layered double hydroxides for removal of oxyanions: A review // Water Res. – 2008. – Vol. 42, N 6-7. – P. 1343-1368. http://dx.doi.org/10.1016/j.watres.2007.10.003

Rives V., Ulibarri M.Layered double hydroxides (LDH) intercalated with metal coordination compounds and oxometalates // Coord. Chem. Rev. – 1999. – Vol. 181, N 1. – P. 61-120. http://dx.doi.org/10.1016/S0010-8545(98)00216-1

Constantino V., Pinnavaia T.Basic properties of Mg2+1-xAl 3+xlayered double hydroxides intercalated by carbonate, hydroxide, chloride, and sulfate anions // Inorg. Chem. – 1995. – Vol. 34, N 4. – P. 883-892. http://dx.doi.org/10.1021/ic00108a020

Geng C., Xu T., Li Y., Chang Z., Sun X.Effect of synthesis method on selective adsorption of thiosulfate by calcined MgAl-layered double hydroxides // Chem. Eng. J. – 2013 –Vol. 232. –P. 510-518. http://dx.doi.org/10.1016/j.cej.2013.08.010

Gonzalez-Pleiter M., Gonzalo S., Rodea-Palomares I., Leganes, F., Rosal, R., Boltes K., Marco E., Fernandez-Pinas F. Toxicity of five antibiotics and their mixtures towards photosynthetic aquatic organisms: Implications for environmental risk assessment // Water Res. – 2013. – Vol. 47, N 6. – P. 2050-2064. http://dx.doi.org/10.1016/j.watres.2013.01.020

Jeong J., Song W., Cooper W., Jung J., Greaves J.Degradation of tetracycline antibiotics: mechanisms and ki-netic studies for advanced oxidation/reduction processes. // Chemosphere. – 2010. – Vol. 78, N 5. – P. 533 – 540. http://dx.doi.org/10.1016/j.chemosphere.2009.11.024

Homem V., Santos L.Degradation and removal methods of antibiotics from aqueous matricese – A review // J. Environ. Managem. – 2011. – Vol. 92, N 10. – P. 2304-2347. http://dx.doi.org/10.1016/j.jenvman.2011.05.023

Li C., Wei M., Evans D., Duan X.Recent advances for layered double hydroxides (LDHs) materials as catalysts applied in green aqueous media // Catal. Today. – 2015 – Vol. 247. – P. 163-169. http://dx.doi.org/10.1016/j.cattod.2014.05.032

Xu Z., Fan J., Zheng S., Ma F., Yin D.On the adsorption of tetracycline by calcined magnesium-aluminum hydrotalcites // J. Environ. Qual. – 2009 – Vol. 38, N 3. – P. 1302-1310. http://dx.doi.org/10.2134/jeq2008.0246

Zhang Y., Hao X., Kuang X, Zhao H., Wen Z. Preparation, characterization and dye adsorption of Au nanopar-ticles/ZnAl layered double oxides nanocomposites // Appl. Surf. Sci. – 2013. – Vol. 283. – P. 505-534. http://dx.doi.org/10.1016/j.apsusc.2013.06.136

Morimoto K., Anraku,C., Hoshino,J., Sato T.Surface complexation reactions of inorganic anions on hydrotalcite-like compounds // J. Colloid Interface Sci. – 2012. – Vol. 384, N 9. – P. 99-104. http://dx.doi.org/d10.1016/j.jcis.2012.06.072

Alanis C., Natividada R., Barrera-Diaz C., Martínez-Mirandab V., Prince J., Valente J. Photocatalytically en-hanced Cr(VI) removal by mixed oxides derived from MeAl (Me:Mg and/or Zn) layered double hydroxides // Appl. Catalysis B. –2013. – Vol.140-141. – P. 546- 551. http://dx.doi.org/10.1016/j.apcatb.2013.04.053

Figueroa R., Leonard A., Mackay A.Modeling tetracycline antibiotic sorption to clays // Environ. Sci. Technol. – 2004. – Vol. 38, N 2. – P. 476-483. http://dx.doi.org/10.1021/es0342087

Chang P., Zhaohui Li, Zh., Jean J.-Sh., Jiang W.-T., Wang Ch.-J., Lin K.-H.Adsorption of tetracycline on 2:1 layered non-swelling clay mineral illite // Appl. Clay Sci. – 2012. – Vol. 67-68. – P. 158–163. http://dx.doi.org/10.1016/j.clay.2011.11.004

Aly A., Osman A., El-Maali N., Al-Hazmi G.Thermal decomposition of tetracycline and cephalosporins metal complexes // Bull. Pharm. Sci., Assiut University. – 2005. – Vol. 28, N 2. – P. 269-276.

Reichle W., Kang S., Everhardt D.The nature of the thermal decomposition of a catalytically active anionic clay mineral // J. Catal. – 1986. – Vol. 101, N 2. –P. 352-359. http://dx.doi.org/10.1016/0021-9517(86)90262-9

Gu C., Karthikeyan K. G.Interaction of tetracycline with aluminum and iron hydrous oxides // Environ. Sci. Technol. – 2005. – Vol. 39, N 8. – P.2660-2667. http://dx.doi.org/10.1021/es048603o

Starukh G.Study of tetracycline adsorption by Zn-Al mixed oxides and layered double hydroxides // Chemistry, Physics and Technology of Surface – 2015. – Vol. 6, N 2. – P. 169-178.

Trujillano R., Holgado M.J., Rives V.Cu-Al-Fe layered double hydroxides with CO32–and anionic surfactants with different alkyl chains in the interlayer // Solid State Sci. – 2005. –Vol. 7, N 8. – P. 931-935. http://dx.doi.org/10.1016/j.solidstatesciences.2005.03.003

Feng Y., Li D., Wang Y., Evans D., Duan X.Synthesis and characterization of a UV absorbent-intercalated Zn-Al layered double hydroxide // Pol. Deg. Stab. – 2006. – Vol. 91, N 4. – P.789-794. http://dx.doi.org/10.1016/j.polymdegradstab.2005.06.006

Myers H., Tochon-Danguy H., Baud C.IR absorption spectrophotometric analysis of the complex formed by tetracycline and synthetic hydroxyapatite // Calcif. Tissue Int. – 1983. – Vol. 35, N 1. – P. 745-749. http://dx.doi.org/10.1007/BF02405117


Пристатейна бібліографія ГОСТ


1.  Cavani F.,Trifirò F., Vaccari A.Hydrotalcite-type anionic clays: Preparation, properties and applications // Catal. Today. – 1991 – Vol. 11, N 2. – P. 173-301. http://dx.doi.org/10.1016/0920-5861(91)80068-K

 

2.  Xu R., Pang W., Huo Q. Modern Inorganic Synthetic Chemistry [Assembly chemistry of anion-intercalated layered materials]. Amsterdam, Elsevier, 2011. 590p.

 

3.  Abelló S., Medina F., Tichit D., Pérez-Ramírez J., Groen J., Sueiras J., Salagre P., Cesteros Y.Aldol Condensations Over Reconstructed Mg–Al Hydrotalcites: Structure–Activity Relationships Related to the Rehydration Method // Chem. Eur. J. – 2005 – Vol. 11, N 2. – P. 728-739. http://dx.doi.org/10.1002/chem.200400409.

 

4.  Del Hoyo C.Layered double hydroxides and human health: An overview // Appl. Clay Sci. – 2007 – Vol. 36, N 1-3. – P. 103-121. http://dx.doi.org/10.1016/j.clay.2006.06.010

 

5.  Vaccari A.Clays and catalysis: a promising future // Appl. Clay Sci. – 1999. – Vol. 14, N 3. – P.161–198.

 

6.  Goh K., Lim T., Gong Z. Application of layered double hydroxides for removal of oxyanions: A review // Water Res. – 2008. – Vol. 42, N 6-7. – P. 1343-1368. http://dx.doi.org/10.1016/j.watres.2007.10.003

 

7.  Rives V., Ulibarri M.Layered double hydroxides (LDH) intercalated with metal coordination compounds and oxometalates // Coord. Chem. Rev. – 1999. – Vol. 181, N 1. – P. 61-120. http://dx.doi.org/10.1016/S0010-8545(98)00216-1

 

8.  Constantino V., Pinnavaia T.Basic properties of Mg2+1-xAl 3+xlayered double hydroxides intercalated by carbonate, hydroxide, chloride, and sulfate anions // Inorg. Chem. – 1995. – Vol. 34, N 4. – P. 883-892. http://dx.doi.org/10.1021/ic00108a020

 

9.  Geng C., Xu T., Li Y., Chang Z., Sun X.Effect of synthesis method on selective adsorption of thiosulfate by calcined MgAl-layered double hydroxides // Chem. Eng. J. – 2013 –Vol. 232. –P. 510-518. http://dx.doi.org/10.1016/j.cej.2013.08.010

 

10.  Gonzalez-Pleiter M., Gonzalo S., Rodea-Palomares I., Leganes, F., Rosal, R., Boltes K., Marco E., Fernandez-Pinas F. Toxicity of five antibiotics and their mixtures towards photosynthetic aquatic organisms: Implications for environmental risk assessment // Water Res. – 2013. – Vol. 47, N 6. – P. 2050-2064. http://dx.doi.org/10.1016/j.watres.2013.01.020

 

11.  Jeong J., Song W., Cooper W., Jung J., Greaves J.Degradation of tetracycline antibiotics: mechanisms and ki-netic studies for advanced oxidation/reduction processes. // Chemosphere. – 2010. – Vol. 78, N 5. – P. 533 – 540. http://dx.doi.org/10.1016/j.chemosphere.2009.11.024

 

12.  Homem V., Santos L.Degradation and removal methods of antibiotics from aqueous matricese – A review // J.  Environ. Managem. – 2011. – Vol. 92, N 10. – P. 2304-2347. http://dx.doi.org/10.1016/j.jenvman.2011.05.023

 

13.   Li C., Wei M., Evans D., Duan X.Recent advances for layered double hydroxides (LDHs) materials as catalysts applied in green aqueous media // Catal. Today. – 2015 – Vol. 247. – P. 163-169. http://dx.doi.org/10.1016/j.cattod.2014.05.032

 

14.  Xu Z., Fan J., Zheng S., Ma F., Yin D.On the adsorption of tetracycline by calcined magnesium-aluminum hydrotalcites // J. Environ. Qual. – 2009 – Vol. 38, N 3. – P. 1302-1310. http://dx.doi.org/10.2134/jeq2008.0246

 

15.  Zhang Y., Hao X., Kuang X, Zhao H., Wen Z. Preparation, characterization and dye adsorption of Au nanopar-ticles/ZnAl layered double oxides nanocomposites // Appl. Surf. Sci. – 2013. – Vol. 283. – P. 505-534. http://dx.doi.org/10.1016/j.apsusc.2013.06.136

 

16.  Morimoto K., Anraku,C., Hoshino,J., Sato T.Surface complexation reactions of inorganic anions on hydrotalcite-like compounds // J. Colloid Interface Sci. – 2012. – Vol. 384, N 9. – P. 99-104. http://dx.doi.org/d10.1016/j.jcis.2012.06.072

 

17.  Alanis C., Natividada R., Barrera-Diaz C., Martínez-Mirandab V., Prince J., Valente J. Photocatalytically en-hanced Cr(VI) removal by mixed oxides derived from MeAl (Me:Mg and/or Zn) layered double hydroxides // Appl. Catalysis B. –2013. – Vol.140-141. – P. 546- 551. http://dx.doi.org/10.1016/j.apcatb.2013.04.053

 

18.  Figueroa R., Leonard A., Mackay A.Modeling tetracycline antibiotic sorption to clays // Environ. Sci. Technol. – 2004. – Vol. 38, N 2. – P. 476-483. http://dx.doi.org/10.1021/es0342087

 

19.  Chang P., Zhaohui Li, Zh., Jean J.-Sh., Jiang W.-T., Wang Ch.-J., Lin K.-H.Adsorption of tetracycline on 2:1 layered non-swelling clay mineral illite // Appl. Clay Sci. – 2012. – Vol. 67-68. – P. 158–163. http://dx.doi.org/10.1016/j.clay.2011.11.004

 

20.  Aly A., Osman A., El-Maali N., Al-Hazmi G.Thermal decomposition of tetracycline and cephalosporins metal complexes // Bull. Pharm. Sci., Assiut University. – 2005. – Vol. 28, N 2. – P. 269-276.

 

21.  Reichle W., Kang S., Everhardt D.The nature of the thermal decomposition of a catalytically active anionic clay mineral // J. Catal. – 1986. – Vol. 101, N 2. –P. 352-359. http://dx.doi.org/10.1016/0021-9517(86)90262-9

 

22.  Gu C., Karthikeyan K. G.Interaction of tetracycline with aluminum and iron hydrous oxides // Environ. Sci. Technol. – 2005. – Vol. 39, N 8. – P.2660-2667. http://dx.doi.org/10.1021/es048603o

 

23.  Starukh G.Study of tetracycline adsorption by Zn-Al mixed oxides and layered double hydroxides // Chemistry, Physics and Technology of Surface – 2015. – Vol. 6, N 2. – P. 169-178.

 

24.  Trujillano R., Holgado M.J., Rives V.Cu-Al-Fe layered double hydroxides with CO32–and anionic surfactants with different alkyl chains in the interlayer // Solid State Sci. – 2005. –Vol. 7, N 8. – P. 931-935. http://dx.doi.org/10.1016/j.solidstatesciences.2005.03.003

 

25.  Feng Y., Li D., Wang Y., Evans D., Duan X.Synthesis and characterization of a UV absorbent-intercalated Zn-Al layered double hydroxide // Pol. Deg. Stab. – 2006. – Vol. 91, N 4. – P.789-794. http://dx.doi.org/10.1016/j.polymdegradstab.2005.06.006

 

26.  Myers H., Tochon-Danguy H., Baud C.IR absorption spectrophotometric analysis of the complex formed by tetracycline and synthetic hydroxyapatite // Calcif. Tissue Int. – 1983. – Vol. 35, N 1. – P. 745-749. http://dx.doi.org/10.1007/BF02405117




DOI: https://doi.org/10.18524/2304-0947.2015.3(55).56248

Посилання

  • Поки немає зовнішніх посилань.


Creative Commons License
Ця робота ліцензована Creative Commons Attribution-ShareAlike 4.0 International License.