МЕХАНІЗМИ ФОРМУВАННЯ НА ПОРИСТИХ НОСІЯХ КОМПЛЕКСІВ d МЕТАЛІВ ТА ЇХ КАТАЛІТИЧНА АКТИВНІСТЬ В РЕДОКС-РЕАКЦІЯХ
DOI:
https://doi.org/10.18524/2304-0947.2015.2(54).50626Ключові слова:
carbon monoxide, phosphine, ozone, sulfur dioxide, redox reactions, supported metal-complex catalysts.Анотація
В огляді узагальнено праці авторів в галузі створення закріплених на пористих носіях різного походження металокомплексних каталізаторів редокс-реакцій за участю фосфіну, монооксиду вуглецю, озону та діоксиду сірки. Проаналізовано фактори, що впливають на механізм формування та склад поверхневих комплексів, а також їх каталітичну активність.Посилання
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Rakitskaya T.L., Reznik L.I., Kiose T.A., Ennan A.A., Hitrich V.F. Rentgenofazovoe issledovanie zakreplennogo na bazal'tovom tufe Pd(II)-Su(II)-katalizatora [X-ray phase investigation of a basalt tuff anchored Pd(II)-Cu(II) catalyst]. Visn. Odes'k. nac. un-tu. Himija, 2007, vol. 12, no. 2, pp. 99-110 (in Russian).
Rakitskaya T.L., Kiose T.A., Volkova V.Ja. Adsorbcionnye svojstva bazal'tovogo tufa i kataliticheskaja aktivnost' zakreplennyh na nem acidokompleksov v reakcii okislenija monooksida ugleroda [Adsorption prop-erties of basalt tuff and catalytic activity of basalt tuff anchored acido complexes in the reaction of carbon monoxide oxidation]. Ukr. him. zhurn., 2008, vol. 74, no.3-4, pp. 80-85 (in Russian).
Rakitskaya T.L., Kiose T.A., Volkova V.Ja., Barbul O.L. Obg'runtuvannja sposobu oderzhannja katalizatora na osnovi Pd(II), Cu(II) i bazal'tovogo tufu dlja nyz'kotemperaturnogo okysnennja monooksydu vuglecju kysnem [Foundation of a method for obtaining based on Pd(II), Cu(II) and basalt tuff catalyst for carbon monoxide oxidation with oxygen]. Visn. Odes'k. nac. un-tu. Himija, 2008, vol. 13, no. 11, pp. 5-14 (in Ukrainian).
Rakitskaya T.L,Kiose T.A., Voloshchuk L.P., Oleksenko L.P., Volkova V.Ja., Reznik L.I. Vlijanie kislotnogo modificirovanija bazal'tovogo tufa na kataliticheskuju aktivnost' zakreplennyh acidokompleksov palladija(II) imedi(II) v reakcii okislenija monooksida ugleroda kislorodom vozduha [The influence of acid modification ofbasalt tuff on the catalytic activity of palladium(II) and copper(II) acido complexes anchored on it in the reaction of carbon monoxide oxidation with air oxygen]. Zhurn. priklad. himii, 2009, vol. 82, no. 2, pp. 204-208(in Russian).
Rakitskaya T.L,Kiose T.A., Volkova V.Ja., Ennan A.A. Ispol'zovanie prirodnyh aljumosilikatov Ukrainy dlja razrabotki novyh metallokompleksnyh katalizatorov ochistki vozduha ot gazoobraznyh toksichnyh veshhestv [The use of Ukrainian natural aluminosilicates for the development of new metal-complex catalysts for air purification from gaseous toxicants]. Jenergoteh. resursosber., 2009, no. 6, pp. 18-23 (in Russian)..
Rakitskaya T.L., Vasilechko V.O., Kiose T.A., Grishhuk G.V., Volkova V.Ja. Adsorbcionno-desorbcionnye svojstva bazal'tovyh tufov i kataliticheskaja aktivnost' acidokompleksov palladija(ІІ) i medi(ІІ) v reakcii okislenija oksida ugleroda(ІІ) kislorodom [Adsorption-desorption properties of basalt tuffs and catalytic activity of palladium(II) and copper(II) acido complexes in the reaction of carbon(II) oxide oxidation with oxygen]. Zhurn. priklad. himii, 2010, vol. 83, no. 7, pp. 1079-1084 (in Russian).
Rakyts’ka T.L, Patryljak L.K., Kiose T.O., Volkova V.Ja. Kyslotni ta katalitychni vlastyvosti systemy Pd(II)-Cu(II)-bazal'tovyj tuf [Acidic and catalytic properties of a Pd(II)-Cu(II)-basalt tuff system]. Visn. L'viv. un-tu. Ser. him., 2010, no. 51. pp. 128-134 (in Ukrainian).
Rakyts’ka T.L., Dlubovskij R.M., Kiose T.A., Truba A.S., Oleksenko L.P., Volkova V.Ja. Adsorbcija parov vody prirodnym i himicheski modificirovannym bazal'tovym tufom[Water vapor adsorption by natural and chemically modified basalt tuff].]. Himija, fizyka ta tehnologija poverhni, 2011, vol. 2, no. 1, pp. 76-80 (in Russian).
Rakitskaya T.L., Kiose T.A., Oleksenko L.P., Verbeckaja T.G., Zrjutina A.M., Kameneva A.V. Vlijanie vlagosoderzhanija na aktivnost' zakreplennogo na kislotno-modificirovannom klinoptilolite Pd(II)-Cu(II)–katalizatorav reakcii nizkotemperaturnogo okislenija monooksida ugleroda[The water content influence on the activity of theacid-modifi ed clinoptilolite anchored Pd(II)-Cu(II) catalyst in the reaction of low-temperature carbon monoxide oxidation]. Visn. Odes'k. nac. un-tu. Himija, 2011, vol. 16, no. 4, pp. 5-11 (in Russian).
Rakitskaya T.L., Kiose T.A., Vasylechko V.O. , Volkova V.Y., Gryshhouk G.V. Adsorption-desorption properties of clinoptilolites and the catalytic activity of surface Cu(II)-Pd(II) complexes in the reaction of carbon monoxide oxidation with oxygen. Chem. Metals Alloys, 2011, vol. 4, no. 3-4, pp. 213-218.
Rakitskaya T.L., Kiose T.A., Oleksenko L.P., Lucenko L.V., Dlubovskij R.M., Volkova V.Ja. Vlijanie soderzhanija vody na aktivnost' zakreplennogo na kislotno-modificirovannom bazal'tovom tu�e Pd(II)-Cu(II)–katalizatora okislenija monooksida ugleroda kislorodom[The water content influence on the activity of the acid-modified basalt tuff anchored Pd(II)-Cu(II) catalyst for the low-temperature carbon monoxide oxidation with oxygen]. Zhurn. priklad. himii, 2012, vol. 85, no.9, pp. 1422-1428(in Russian).
Rakitskaya T.L., Kiose T.A., Reznik L.I. Prirodnye i himicheski modificirovannye bazal'tovye tufy. Fazovyj sostav i kataliticheskaja aktivnost' poverhnostnyh Cu(II)-Pd(II)–kompleksov v reakcii okislenija monooksida ugleroda kislorodom[Natural and chem.ically modified basalt tuffs. The phase composition and Cu(II)-Pd(II) complexes in the reaction of carbon monoxide oxidation with oxygen]. Himija, fizyka ta tehnologija poverhni. 2012, vol.3, no. 2, pp. 215-222(in Russian).
Rakits’ka T.L., Kiose T.O., Zryutina G.M., Gladyshevskii R.E., Truba A.S., Vasylechko V.O., Gryschouk G.V., Volkova V.Y., Solid-state catalysts based on bentonites and Pd(II)-Cu(II) complexes for low-temperature carbonmonoxide oxidation. “OMEE-20112”: Proc. Int. Conf.Ukraine, Lviv, 2012, pp. 297-298. http://dx.doi.org/10.1109/omee.2012.6464759
Rakitskaya T.L., Kiose T.A.,Ennan A.A. Zavisimost' zashhitnyh svojstv nizkotemperaturnogo katalizatora ot koncentracii CO i jeffektivnogo vremeni kontakta [The dependence of protective properties of a low-tempera-ture catalyst on CO concentration and the effective retaining time]. Visn. Odes'k. nac. un-tu. Himija, 2013, vol. 18, no. 1 (45), pp. 32-38 (in Russian).
Rakitskaya T.L., Kiose T.A., Volkova V.Y. Dzhiga A.M., Golubchik K.O. Sostojanie i perspektivy razrabotki nizkotemperaturnyhkatalizatorov okislenija monooksida ugleroda respiratornogo naznachenija. І. Metallicheskie katalizatory [The state and prospects of the development of low-temperature catalysts of the respiratory protection purpose for carbon monoxide oxidation. I. Metal catalysts]. Visn. Odes'k. nac. un-tu. Himija, 2013, vol. 18, no. 2 (46), pp. 5-15 (in Russian).
Rakitskaya T.L., Kiose T.A., Ennan A.A., Volkova V.Y. Sostojanie i perspektivy razrabotki nizkotemperaturnyhkatalizatorovokislenija monooksida ugleroda respiratornogo naznachenija. ІІ. Oksidnye i oksidno-metallicheskie katalizatory [The state and prospects of the development of low-temperature catalysts of the respiratory protection purpose for carbon monoxide oxidation. I. Metal oxide and metalmetal oxide catalysts]. Visn. Odes'k. nac. un-tu. Himija, 2013, vol. 18, no. 3 (47), pp. 5-10 (in Russian).
Rakitskaya T.L., Kiose T.A., Zryutina A.M., Gladyshevskii R.E., Truba A.S. , Vasylechko V.O. , Demchenko P.Yu., Gryschouk G.V., Volkova V.Y. Solid-state catalysts based on bentonites and Pd(II)-Cu(II) complexesfor low-temperature carbon monoxide oxidation. Solid State Phenomena, 2013, vol. 200, pp.299-304. http://dx.doi.org/10.4028/www.scientific.net/ssp.200.299
Rakitskaya T.L., Kiose T.A., Dzhiga A.M., Volkova V.Y., Golubchik K.O. Sostojanie i perspektivy razrabotki nizkotemperaturnyhkatalizatorov okislenija monooksida ugleroda respiratornogo naznachenija: ІІІ. Nanesennye metallokompleksnye katalizatory [The state and prospects of the development of low-temperature catalysts of the respiratory protection purpose for carbon monoxide oxidation. I. Supported metal-complex catalysts]. Visn. Odes'k. nac. un-tu. Himija, 2013, vol. 18, no. 4 (48), pp. 5-12 (in Russian).
Rakitskaya T.L., Kiose T.A., Oleksenko L.P. Vlijanie soderzhanija vody na aktivnost' nanesennogo na prirodnyjtrepel palladij-mednogo katalizatora okislenija monooksida ugleroda kislorodom[The water content influenceon the activity of a natural tripoli supported palladium(II)-copper(II) catalyst for the carbon monoxide oxidation with oxygen]. Voprosy khimii i khimicheskoi technologii, 2014, no. 3 (96), pp. 56-60 (in Russian).
Rakitskaya T.L., Kiose T.A., Oleksenko L.P., Djiga A.M., Volkova V.Y. Thermochemical and catalytic properties of modified bentonites. Chemistry, physics and technology of surface,2015, vol. 6, no. 2, pp. 196-202.
Rakitskaya T.L., Bandurko A.Ju., Truba A.S. Kinetika razlozhenija ozona kompleksami medi(ІІ) s immobilizovannymi na ajerosile2-gidrokso-3-metoksibenzal'degidiminom[The kinetics of ozone decomposition with complexes of copper(II) with aerosil immobilized2-hydroxo-3-methoxybenzaldehydeimine]. Visn. Odes'k. nac. un-tu. Himija, 2005, vol. 10, no. 2, pp. 170-179 (in Russian).
Rakitskaya T.L., Truba A.S., Raskola L.A., Bandurko A.Ju., Golub A.A. Vlijanie stroenija adsorbirovannyh na poverhnost' SiO2 kompleksov medi(II) na ih kataliticheskuju aktivnost' v reakcii razlozhenija ozona [The influence of a structure of SiO2 surface adsorbed copper(II) complexes on their catalytic activity in the reaction of ozone decomposition]. Teoret. i jeksperim. himija, 2006, vol. 42, no. 1, pp. 55-60 (in Russian).
Rakitskaya T.L., Bandurko A.Ju., Truba A.S., Raskola L.A., Golub A.A. Kompleksy 3d-metallov s immobilizovannymi na ajerosile2-gidroksi-3-metoksibenzal'iminpropiilom i4-gidroksi-3-metoksibenzal'iminpropiilom vreakcii razlozhenija ozona [Complexes of 3d metals with aerosil immobilized 2-hydroxy-3-methoxybenzaldiminepropyl and4-hydroxy-3-methoxybenzaldiminepropyl in the reaction of ozone decomposition]. Zhurn. obshh. himii, 2006, vol. 76, no. 8, pp. 1320-1325(in Russian).
Rakitskaya T.L., Truba A.S., Bandurko A.Ju. Novye metody sinteza immobilizovannyh na razlichnyh nositeljahkompleksov Cu(II), Co(II) i Mn(II) s osnovanijami Shiffa[New methods for synthesis of complexes of Cu(II), Co(II), and Mn(II) with Schiff bases immobilized on various supportd]. Visn. Odes'k. nac. un-tu. Himija, 2006, vol. 11, no. 1, pp. 14-25 (in Russian).
Rakitskaya T.L., Truba A.S., Samburskij S.E., Koroeva L.V. Sostojanie zakreplennogo na oksidnyh nositeljahgeksametilentetramina i jego kompleksov s Cu(II), Co(II) i Mn(II) [The state of hexamethylenetetramine anchored on oxide supports and its complexes Cu(II), Co(II), and Mn(II)]. Visn. Odes'k. nac. un-tu. Himija, 2007, vol. 12, no. 1, pp. 40-47 (in Russian).
Rakitskaya T.L., Truba A.S., Raskola L.A., Ennan A.A. Nizkotemperaturnye Cu-soderzhashhie katalizatory razlozhenija ozona[Low-temperature Cu containing catalysts for ozone decomposition]. Visn. Odes'k. nac. un-tu. Himija, 2008, vol. 13, no. 2, pp. 73-92 (in Russian).
Rakitskaya T.L., Raskola L.A., Kiose T.A., Zaharija A.N., Kitajskaja V.V. Adsorbcija ionov 3d-metallov prirodnym i kislotno-modificirovannym klinoptilolitom[Adsorption of ions of 3d metals by natural and acid-modifiedclinoptilolite]. Visn. Odes'k. nac. un-tu. Himija, 2010, vol. 15, no. 3, pp. 85-91 (in Russian).
Rakitskaya T.L., Truba A.S., Davtjan A.S., Berezina L.V. Kataliticheskaja aktivnost' zakreplennyh nabazal'tovom tufe hlorokompleksov Cu(II), Co(II)i Mn(II) [The catalytic activity of basalt tuff anchored chloridecomplexes of Cu(II), Co(II), and Mn(II)]. Visn. Odes'k. nac. un-tu. Himija, 2010, vol. 15, no. 1-2, pp. 10-16 (in Russian).
Rakyts’ka T., Ennan A., Raskola L., Truba A., Kytajs’ka V. Nyz’kotemperaturnyj rozklad ozonu zakriplenymy na klynoptyloliti acydokompleksamy Cu(II) [The low-temperature ozone decomposition with clinoptilolite anchored Cu(II) acido complexes]. Visn. L'viv. un-tu. Ser. him., 2010, no. 51. pp. 135-140 (in Ukrainian).
Rakitskaya T.L., Truba A.S., Golub A.A., Radchenko E.A. Razlozhenie ozona immobilizovannymi na ajerosile oksial'diminami[Ozone decomposition with aerosil immobilized oxyaldimines]. Visn. Odes'k. nac. un-tu. Hi-mija, 2010, vol. 15, no. 2, pp. 15-22(in Russian).
Rakitskaya T.L., Truba A.S., Golub A.A., Kiose T.A., Radchenko E.A. Vlijanie sostava i stroenija kompleksov kobal'ta(II) s oksial'diminopropilajerosilami na ih kataliticheskuju aktivnost' v reakcii razlozhenija ozona[The influence of the composition and structure of complexes of cobalt(II) with oxyaldiminepropyl aerosils on their catalytic activity in the reaction of ozone decomposition]. Teoret. i jeksperim. himija, 2011, vol. 47, no. 5, pp. 321-326(in Russian).
Rakitskaya T.L., Raskola L.A., Truba A.S., Kiose T.A., Reznik L.I. Kataliticheskoe razlozhenie ozona zakreplennymi na prirodnom klinoptilolite acidokompleksami kobal'ta(ІІ) [The catalytic ozone decomposition with natural clinoptilolite anchored cobalt(II) acido complexes]. Voprosy khimii i khimicheskoi technologii, 2011, no. 2, pp. 118-123 (in Russian).
Rakitskaya T.L., Kiose T.A., Dzhiga A.M., Toporov S.V. IK-spektral'noe issledovanie struktury i fazovogo sostava bentonitov Ukrainy[The IR study of the structure and phase composition of Ukrainian bentonites]. Visn. Odes'k. nac. un-tu. Himija, 2012, vol. 17, no. 1 (41), pp. 13-19 (in Russian).
Rakitskaya T.L., Truba A.S., Kiose T.A., Berezina L.V., Davtjan A.S. Protolitychni vlastyvosti pryrodnyh ta modyfikovnyh sorbentiv [Protolitic properties of natural and modified sorbents]. Visn. Odes'k. nac. un-tu. Hi-mija, 2012, vol. 17, no. 2 (42), pp. 12-17 (in Ukrainian).
Rakytskaya T.L., Kiose T.A., Truba A.S., Ennan A.A., Dlubovskiy R.M., Volkova V.Y. Adsorption of watervapour by natural and chemically modified clinoptilolite and mordenite samples. Chemistry, physics and tech- , physics and tech- physicsand technology of surface,2012, vol. 3, no. 4, pp. 455-462.
Rakitskaya T.L., Truba A.S., Raskola L.A., Radchenko E.A., Strizhak A.V., Golub A.A. Antiozonantnaja aktivnost' modificirovannyh kompleksami 3d-metallov kremnezemov [The antiozonant activity of silicas modified with3d metals]. Zhurn. obshh. Himii, 2013, vol. 83, no. 2, pp. 305-312(in Russian).
Rakitskaya T.L., Truba A.S., Raskola L.A. Katalizatory nizkotemperaturnogo razlozhenija ozona na osnove hloridov3d-metallov i prirodnyh sorbentov[Catalysts based on chlorides of 3d metals and natural sorbents for the low-temperature ozone decomposition]. Vcheni zapysky Tavrijs'kogo nacional'nogo universytetu im. V.I. Vernads'kogo. Serija„Biologija, himija”, 2013, vol. 26 (65), no.4, pp. 358-371 (in Russian).
Rakitskaya T.L., Truba A.S., Raskola L.A., Ennan A.A. Modificirovannyj hloridom marganca(ІІ) prirodnyj klinoptilolit v reakcii razlozhenija ozona[Natural clinoptilolite modified with manganese(II) chloride in the reaction of ozone decomposition]. Himija, fizyka ta tehnologija poverhni, 2013, vol. 4, no.3, pp. 297-304 (in Russian).
Rakitskaya T.L., Truba A.S., Ennan A.A., Dlubovskij R.M. Adsorbcija parov vody prirodnymi i modifi cirovannymi hloridami marganca(ІІ) i kobal'ta(ІІ) sorbentami[The water vapor adsorption by sorbents, natural and modified with manganese(II) and cobalt(II) chlorides]. Voprosy khimii i khimicheskoi technologii,2014, no.1, pp. 131-135(in Russian).
Rakytskaya T.L., Truba A.S., Kiro S.A., Volkova V.Y. Nanostructured materials based on the solid component of welding aerosol as catalysts for low-temperature ozon decomposition. “OxideMaterials for Electronic Engineering”: Proc. Int. Conf., Ukraine, Lviv, 2014, pp. 230-231. http://dx.doi.org/10.1109/omee.2014.6912425
Rakitskaya T.L., Truba A.S., Ennan А.A., Kiro S.A., Volkova V.Y. Phase composition and catalytic activity of nanostructured materials based on solid component of welding aerosol. Solid State Phenomena, 2015, vol. 230, pp. 279-284. http://dx.doi.org/10.4028/www.scientific.net/ssp.230.279
Rakyts’ka T.L., Kiose T.O, Gavrylenko M.I., Volkova V.Ja., Misharina N.O. Dynamika sorbcii’ dioksydu sirky bazal’tovym tufom [The dynamics of sulfur dioxide sorption by basalt tuff]. Visn. Odes'k. nac. un-tu. Himija, 2006, vol. 11, no. 4, pp. 5-12 (in Ukrainian).
Rakyts’ka T.L., Kiose T.O., Gavrylenko M.I., Postalatij O.M. Nyz’kotemperaturne okysnennja dioksydu sirky v prysutnosti zakriplenogo na bazal’tovomu tufi hlorydu kuprumu(II) [The low-temperature sulfur dioxide oxidation over basalt tuff anchored copper(II) chloride]. “L'vivs'ki himichni chytannja”: Zb. nauk. prac' 11nauk. konf. [“L'vivchemical readings”: Collected scientific papers of 11th Sci. Conf.]. Ukraine, L'viv, 2007, p. T4 (in Ukrainian).
Gavrylenko M.I., Kiose T.O., Rakitskaya T.L., Postalatij O.M. Sorbcyja dyoksyda sery bazal'tovym tufom, impregnirovannymvodnym rastvorom geksametilentetramina [The sul�fur dioxide sorption by basalt tuff impregnated withhexamethylenetetramine aqueous solution]. Visn. Odes'k. nac. un-tu. Himija, 2008, vol. 13, no. 12, pp. 79-84(in Russian).
Rakyts’ka T.L., Kiose T.O., Kamenjeva O.V., Myhajlova O.V. Adsorbcijni vlastyvosti pryrodnyh sorbentiv vidnosno dioksydu sirky [Adsorption properties of natural sorbents with respect to sulfur dioxide]. Visn. Odes'k. nac. un-tu. Himija, 2011, vol. 16, no. 14, pp. 91-94 (in Ukrainian).
Rakitskaya T.L., Kiose T.A., Kameneva Je.V., Jarych A.V., Volkova V.Ja. Modificyrovannye ionami medi(II) pryrodnye sorbenty v reakcii nizkotemperaturnogo okyslenija dioksida sery[Natural sorbents modified with copper(II) ions in the reaction of sulfur dioxide oxidation]. Vchenizapysky Tavrijs'kogo nacional'nogo universytetu im. V.I. Vernads'kogo. Serija„Biologija, himija”, 2013, vol. 26 (65), no.4, pp. 345-357 (in Russian).
Rakitskaya T.L., Raskola L.A., Kiose T.A., Jarchuk A.V., Korotkova A.S. Adsorbcionnye i zashhitnye svojstva modificirovannogo klinoptilolita otnositel'no dioksida sery[Adsorption and protective properties of modified clinoptilolite with respect to sulfur dioxide]. Visn. Odes'k. nac. un-tu. Himija, 2014, vol. 19, no. 1 (49), pp. 49-56 (in Russian).
Rakitskaya T.L., Kiose T.A., Kameneva Je.V. Adsorbcionnye svojstva prirodnyh sorbentov otnositel'no dioksida sery i parov vody[Adsorption properties of natural sorbents with respect to sulfur dioxide]. Himija, fizyka ta tehnologija poverhni.2014, vol. 5, no. 1, pp. 56-63 (in Russian).
Rakytskaya T.L., Kameneva E.V., Kiose T.A., Volkova V.Y. Solid-state compositions for low-temperature sulfur dioxide oxidation consisting of natural clinoptilolite, copper(II) and halide ions. “OMEE-20112”:Proc. Int. Conf. Ukraine, Lviv, 2012, pp. 228-229. http://dx.doi.org/10.4028/www.scientific.net/ssp.200.299
Rakitskaya T.L., Kiose T.A., Kameneva E.V., Volkova V.Y. Natural clinoptilolite based solid-state compositions for low-temperature air purification from sulphur dioxide. Solid State Phenomena, 2015, vol. 230, pp.291-296. http://dx.doi.org/10.4028/www.scientific.net/ssp.230.291
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